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91.
Electron Loss Spectroscopy (ELS), X-ray Photoemission (XPS), Secondary Emission Energy Distribution, and Secondary Electron yield data have been obtained on both evaporated films and sprayed-on coatings of BaO. Using the ELS correlated with the XPS data, bulk and surface plasmon losses as well as excitonic and interband transition electron loss mechanisms have been identified. It was found that at low primary beam energies (<100 eV), structure in the secondary emission energy distribution could be correlated with a conduction band energy structure. This structure was consistent with the model used to explain the loss transitions. The structure in the energy distribution curves shows little, if any, correlation with plasmon decay mechanisms and other two-step electron emission processes. On the contrary, for the case of BaO (at least at low primary energies), the energy distribution data and structure in the secondary yield vs. primary beam energy data indicate that most secondaries are produced by direct excitation of secondaries by the primary electrons. 相似文献
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H. Hübel R. M. Diamond P. Aguer C. Ellegaard D. B. Fossan H. Kluge C. Schück S. Shih F. S. Stephens U. Smilanski 《Zeitschrift für Physik A Hadrons and Nuclei》1982,304(3):225-230
Average lifetimes of unresolved transitions deexciting very high spin states populated in28Si(136, 129Xe,xn)164? x, 157?xEr reactions have been determined by a Doppler shift attenuation method. We find that the yrast bump region between 1.0 and 1.6 MeV contains a majority of strongly collectiveE2 transitions with very short lifetimes (a few tens of fsec) in the well deformed nuclei around159Er and, with less certainty, almost comparably short lifetimes in the more spherical nuclei around152Er. In the high energy region of 2.0–3.2 MeV we observe transitions which depopulate longer lived states in the nuclei nearN=82 than in the well deformed systems. 相似文献
95.
Ab initio SCF and CI calculations are reported which find the cyclic conformer of ozone to lie 16 kcal/mole above the preferred (open-chain) form of this substance. Polarization functions in the AO basis set are found to be quite important in this determination, strongly favoring the cyclic species. The possible experimental significance of such a relatively stable ring conformer of ozone is assessed. 相似文献
96.
The concept of coefficient shift matrix is introduced to represent delay variables in block pulse series. The optimal control of a linear delay system with quadratic performance index is then studied via block pulse functions, which convert the problems into the minimization of a quadratic form with linear algebraic equation constraints. The solution of the two-point boundary-value problem with both delay and advanced arguments is circumvented. The control variable obtained is piecewise constant. 相似文献
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Total syntheses of 1α- and 1β-methyl thienamycin are reported. 1β-Methyl thienamycin retains the antibacterial activity of thienamycin and is highly resistant to hydrolysis by DHP-I enzyme. 相似文献
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Analysis of the plasma emission from a low-pressure microwave cavity discharge through flowing hydrogen peroxide vapor showed that both H and OH were produced in proportions which varied with the applied power. When the dissociated vapor was condensed at 195 K only water was obtained; at 77 K, H2O2 and H2O4 were also obtained. Their formation could not be increased by increasing the H atom or OH radical concentration in the plasma. When the reaction time of the dissociated vapor between the plasma exit and the cold surface was increased, the rate of H2O2 formation increased mostly at the expense of water formation. It appears that, as in the case of the reaction of H with O2, the rate of H2O2 formation is dependent on the concentration of O2 produced in the spatial afterglow by the gas-phase reactions of the hydroxyl radicals. 相似文献